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Novel rearrangements for C-H functionalisation
We have developed new methods for the functionalization of C-H bonds through rearrangement processes. We have developed 1,5 and 1,4 hydride shift and subsequent cyclisation strategies for the functionalisation of C-H bonds adjacent to amines. We have synthesised fused heterocycles using this methodology and used it in a key step for the synthesis of vallesamidine, strempeliopine and schizozygine alkaloids. In addition we are investigating a new sigmatropic process for the functionalization of C-H bonds adjacent to ethers.
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