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Publication Detail
Molecular Auger Interferometry
  • Publication Type:
  • Authors:
    Khokhlova M, Cooper B, Ueda K, Prince KC, Kolorenč P, Ivanov M, Averbukh V
  • Publication date:
  • Published proceedings:
    Journal of Physics: Conference Series
  • Volume:
  • Issue:
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  • Name of conference:
    31st International Conference on Photonic, Electronic and Atomic Collisions (ICPEAC XXXI)
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© 2019 Published under licence by IOP Publishing Ltd. We propose a theory of interferometric measurement of a normal Auger decay width in molecules. Molecular Auger interferometry is based on the coherent phase control of Auger dynamics in a two-colour (ω/2ω) laser field. We show that, in contrast to atoms, in oriented molecules of certain point groups (e.g. CH3F) the relative ω/2ω phase modulates the total ionisation yield. A simple analytical formula is derived for the extraction of the widths of Auger-active states from a molecular Auger interferogram, avoiding the need of either attosecond or high-resolution spectroscopy.
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